Two Studies in Gas-Phase Ion Spectroscopy
Vacuum-Ultraviolet Negative Photoion Spectroscopy and Ion-Molecule Reaction Kinetics
(Sprache: Englisch)
This report covers two investigations into gas-phase ion spectroscopy; the first using tunable vacuum-ultraviolet radiation to identify negative ions from photoexcited polyatomic molecules, and the second studying ion flow tube mass spectrometry.
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This report covers two investigations into gas-phase ion spectroscopy; the first using tunable vacuum-ultraviolet radiation to identify negative ions from photoexcited polyatomic molecules, and the second studying ion flow tube mass spectrometry.
Klappentext zu „Two Studies in Gas-Phase Ion Spectroscopy “
In this thesis Matthew Simpson reportstwo areas of work in gas ion spectroscopy, each investigation in itself worthy of a PhD. The first study uses tunable vacuum-ultraviolet radiation from a synchrotron to identify negative ions from twenty four photoexcited polyatomic molecules in the gas phase. From these experiments, Matthew collects a vast amount of data and summarises and reviews ion-pair formation from polyatomic molecules. The second study is on selected ion flow tube mass spectrometry. Matthew investigates the reactions of cations and anions with ethene, monofluoroethene, 1,1-difluoroethene and tetrafluoroethene. In this study Matthew tries to explain why certain products are formed preferentially over other products at a microscopic level of understanding. The data recorded in this thesis form the most comprehensive collection of information about anion formation and are the basis of a review and numerous articles in specialist journals.
Inhaltsverzeichnis zu „Two Studies in Gas-Phase Ion Spectroscopy “
Introduction and background information.- The experiments.- Vacuum-ultraviolet negative photoion spectroscopy of SF6, CF4 and SF5CF3.- Vacuum-ultraviolet negative photoion spectroscopy of CF3Cl, CF3Br and CF3I.- Vacuum-ultraviolet negative photoion spectroscopy of SF5Cl.- Vacuum-ultraviolet negative photoion spectroscopy of small polyatomic molecules.- The reactions of CFn+ (n = 1-3) with C2H4, C2H3F, CH2CF2 and C2HF3.- The reactions of C2F4+ with C2H4, C2H3F, CH2CF2 and C2HF3.- Reactions of OH-, O-, CF3-, F- and O2- with C2H4, C2H3F, CH2CF2, C2HF3 and C2F4 .
Bibliographische Angaben
- Autor: Matthew J. Simpson
- 2013, 2012, XIV, 162 Seiten, Masse: 15,5 x 23,5 cm, Kartoniert (TB), Englisch
- Verlag: Springer, Berlin
- ISBN-10: 3642271278
- ISBN-13: 9783642271274
Sprache:
Englisch
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